Which word is synonymous with 'to cause irritation or anger'?

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The term that best captures the idea of 'to cause irritation or anger' includes both "vex" and "rankle."

"Vex" specifically means to irritate or annoy someone, often in a way that provokes frustration. It conveys a sense of mental distress or trouble, making it an apt choice for expressing irritation.

"Rankle," on the other hand, suggests a deeper, more persistent source of irritation or resentment. When something rankles, it causes ongoing discomfort or anger, often indicating a wound that has not healed or a grievance that continues to bother someone.

Both words effectively communicate different nuances of causing irritation or anger, making the combined choice of both "vex" and "rankle" the correct answer.